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Environmental Chemistry publishes papers reporting chemistry that enhances our understanding of the environment including air, water, soil, sediments, and biota. More

Editor-in-Chief: Kevin Francesconi

 
 
 

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Published online 25 September 2014
Long term PM2.5 trends in the Australian industrial city of Newcastle: a 15-year study from 1998 to 2013 
Eduard Stelcer, David D. Cohen and Armand J. Atanacio

Environmental context. Long-term exposure to fine particle air pollution has significant implications for human health. At a mixed urban–industrial site in Newcastle, Australia, we identified contributions from individual industrial aerosol sources in addition to the more common aerosol sources such as soil, sea and smoke. These results are significant for the assessment and management of fine particulate air pollution in the Newcastle air shed.

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Published online 15 September 2014
Dissolution of metal and metal oxide nanoparticles under natural freshwater conditions 
Niksa Odzak, David Kistler, Renata Behra and Laura Sigg

Environmental context. Engineered nanomaterials (e.g. silver, zinc oxide and copper oxide) are being widely used in many consumer products such are cosmetics, food packaging and textiles. During their usage and treatment, they will be released to natural waters and partly dissolve, depending on the water type and nanomaterial characteristics. These nanomaterials may thus have some toxic effects to aquatic organisms and indirectly to humans because of higher concentrations of dissolved silver, zinc and copper in natural waters.

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    | Supplementary Material (508 KB)
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Published online 05 September 2014
Voltammetric study of an FeS layer on a Hg electrode in supersaturated FeS chloride solution 
D. Krznarić and I. Ciglenečki

Environmental context. During the electrochemical analysis of natural waters, the Hg electrode could become the site for surface metal sulfide formation, such as FeS, which can have significant influence on the voltammetric determination of FeII. Reduction of FeII in such conditions can occur both on the bare Hg surface and on the FeS-modified Hg surface. Until recently, measurements of FeII have considered only the signal obtained from reduction on the bare Hg surface, and hence may have underdetermined the true FeII content of natural samples.

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Published online 08 August 2014
In vitro cytotoxicity assessment of a hydraulic fracturing fluid 
Madeleine E. Payne, Heather F. Chapman, Janet Cumming and Frederic D. L. Leusch

Environmental context. Hydraulic fracturing fluids, used in large volumes by the coal seam gas mining industry, are potentially present in the environment either in underground formations or in mine wastewater (produced water). Previous studies of the human health and environmental effects of this practice have been limited because they use only desktop methods and have not considered combined mixture toxicity. We use a novel in vitro method for toxicity assessment, and describe the toxicity of a hydraulic fracturing fluid on a human gastrointestinal cell line.

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    | Supplementary Material (149 KB)
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Published online 20 June 2014
Microbial fuel cells under extreme salinity: performance and microbial analysis 
Oihane Monzon, Yu Yang, Cong Yu, Qilin Li and Pedro J. J. Alvarez

Environmental context. The treatment of extremely saline, high-strength wastewaters while producing electricity represents a great opportunity to mitigate environmental effects and recover resources associated with wastes from shale oil and gas production. This paper demonstrates that extreme halophilic microbes can produce electricity at salinity up to 3- to 7-fold higher than sea water.

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blank image Environmental Chemistry
Volume 11 Number 5 2014
RESEARCH FRONT: Arsenic Biogeochemistry and Health

 
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Foreword to the Research Front on ‘Arsenic Biogeochemistry and Health' 
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Andreas Kappler
pp. i-i
 
 

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Arsenic mobility and toxicity in South and South-east Asia – a review on biogeochemistry, health and socio-economic effects, remediation and risk predictions 
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E. Marie Muehe and Andreas Kappler
pp. 483-495

Environmental context. The presence of high arsenic concentrations in South and South-east Asian groundwater causes dramatic health issues for the local population. As a consequence, scientists, governments and agencies investigate arsenic-related health issues and arsenic origin, fate and behaviour in ground- and drinking water and have started to provide remediation and mitigation strategies. This review broadly summarises our current knowledge on arsenic biogeochemistry, health and socio-economic effects, remediation and risk predications in Asia and discusses current and future research directions.

 
  
 

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Arsenic cycling in freshwater phytoplankton and zooplankton cultures 
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G. Caumette , I. Koch , K. House and K. J. Reimer
pp. 496-505

Environmental context. Understanding how arsenic is changed from toxic to non-toxic chemical forms in lakes and rivers is important in understanding the overall risk from arsenic. Freshwater plankton exposed in laboratory cultures to different sources of toxic inorganic arsenate formed arsenosugars, but at higher exposure levels, in water and through contaminated sediment, inorganic arsenate remained unchanged. In arsenic-contaminated freshwater bodies, plankton may provide a source of toxic inorganic arsenic to consumers.

 
    | Supplementary Material (665 KB)
 

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Biosynthesis of arsenolipids by the cyanobacterium Synechocystis sp. PCC 6803 
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Xi-Mei Xue , Georg Raber , Simon Foster , Song-Can Chen , Kevin A. Francesconi and Yong-Guan Zhu
pp. 506-513

Environmental context. Arsenic biotransformation processes play a key role in the cycling of arsenic in aquatic systems. We show that a freshwater cyanobacterium can convert inorganic arsenic into arsenolipids, and the conversion efficiency depends on the arsenic concentration. The role of these novel arsenic compounds remains to be elucidated.

   | Supplementary Material (388 KB)  |        Open Access Article
 

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Release of arsenite, arsenate and methyl-arsenic species from streambed sediment affected by acid mine drainage: a microcosm study 
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Marina Héry , Corinne Casiot , Eléonore Resongles , Zoe Gallice , Odile Bruneel , Angélique Desoeuvre and Sophie Delpoux
pp. 514-524

Environmental context. Arsenic-rich waters generated from the oxidation of mining wastes are responsible for the severe contamination of river waters and sediments located downstream from mining sites. Under certain environmental conditions, the affected riverbed sediments may represent a reservoir for arsenic from which this toxic element may be released into water, mainly as a consequence of microbial activity.

 
    | Supplementary Material (536 KB)
 

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In situ oxalic acid injection to accelerate arsenic remediation at a superfund site in New Jersey 
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Karen Wovkulich , Martin Stute , Brian J. Mailloux , Alison R. Keimowitz , James Ross , Benjamin Bostick , Jing Sun and Steven N. Chillrud
pp. 525-537

Environmental context. Arsenic is one of the most common contaminants at US Superfund sites; therefore, establishing techniques to accelerate As remediation could benefit many sites. In a pilot scale study, we determined that addition of oxalic acid to the subsurface has the potential to increase arsenic release from sediments and possibly improve remediation efficiency by pump and treat techniques. Because pump and treat remediation can require many decades to sufficiently decrease contaminant levels, methods for improving remediation could lead to substantial savings in time and resources.

 
    | Supplementary Material (971 KB)
 

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Microbially mediated reduction of FeIII and AsV in Cambodian sediments amended with 13C-labelled hexadecane and kerogen 
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Athanasios Rizoulis , Wafa M. Al Lawati , Richard D. Pancost , David A. Polya , Bart E. van Dongen and Jonathan R. Lloyd
pp. 538-546

Environmental context. The use of groundwater with elevated concentrations of arsenic for drinking, cooking or irrigation has resulted in the worst mass poisoning in human history. This study shows that organic compounds that can be found in arsenic rich subsurface sediments may be used by indigenous microorganisms, contributing to the release of arsenic from the sediments into the groundwater. This study increases our understanding of the range of organic substrates (and their sources) that can potentially stimulate arsenic mobilisation into groundwaters.

   | Supplementary Material (405 KB)  |        Open Access Article
 

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Factors affecting arsenic and uranium removal with zero-valent iron: laboratory tests with Kanchan-type iron nail filter columns with different groundwaters 
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Christine B. Wenk , Ralf Kaegi and Stephan J. Hug
pp. 547-557

Environmental context. Tens of millions of people worldwide depend on groundwater with naturally high arsenic concentrations for drinking and cooking. We studied simple filters built with locally available and inexpensive iron nails, which can oxidise and bind arsenic in forming iron oxides and rust layers. Filters containing iron are being successfully applied in several regions, but efficiencies depend on the type of groundwater, and sufficiently large iron surfaces and contact times with water are needed for good arsenic removal.

 
    | Supplementary Material (904 KB)
 

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Effectiveness of various sorbents and biological oxidation in the removal of arsenic species from groundwater 
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Anna Corsini , Lucia Cavalca , Gerard Muyzer and Patrizia Zaccheo
pp. 558-565

Environmental context. Arsenic contamination of aquifers is a worldwide public health concern and several technologies have been developed to reduce the arsenic content of groundwater. We investigated the efficiency of various materials for arsenic removal from groundwater and found that iron-based sorbents have great affinity for arsenic even if groundwater composition can depress their ability to bind arsenic. Moreover, we showed that the use of microorganisms can enhance the removal of arsenic from groundwater.

 
  
 

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Solid-phase characterisation of an effective household sand filter for As, Fe and Mn removal from groundwater in Vietnam 
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Andreas Voegelin , Ralf Kaegi , Michael Berg , Katja Sonja Nitzsche , Andreas Kappler , Vi Mai Lan , Pham Thi Kim Trang , Jörg Göttlicher and Ralph Steininger
pp. 566-578

Environmental context. Household sand filters are widely used in Vietnam to remove As, Fe and Mn from groundwater used as drinking water. From the solid-phase characterisation of a sand filter that has been used for 8 years, we conclude that As and Fe are retained by a combination of fast sorption reactions, surface-catalysed Fe oxidation and mediated As co-oxidation and that microbial processes are probably involved in effective Mn retention. This study contributes to a better mechanistic understanding of filter functioning as a basis for further improvements in filter design and operation.

 
    | Supplementary Material (1.2 MB)
 

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Deciphering and predicting spatial and temporal concentrations of arsenic within the Mekong Delta aquifer 
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Benjamin D. Kocar , Shawn G. Benner and Scott Fendorf
pp. 579-594

Environmental context. Himalayan derived arsenic contaminates groundwater across Asia, ranging from the deltas of Ganges-Brahmaputra of Bangladesh to the interior basins of the Yangtze and Yellow Rivers in China, where more than one hundred million people are drinking water with hazardous levels of the toxin. Our ability to predict the distribution and changes in arsenic concentration in aquifers of affected regions has been limited. Here we provide a dynamic model that captures arsenic migration and can be used to forecast changes in groundwater arsenic concentrations.

 
    | Supplementary Material (1.9 MB)
 

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Improved groundwater geogenic arsenic hazard map for Cambodia 
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C. Sovann and D. A. Polya
pp. 595-607

Environmental context. Groundwater arsenic is a major environmental risk to human health in many regions of the world, including Cambodia where groundwater is often used for drinking water. We present data for hitherto poorly sampled regions in Cambodia, notably around Tonle Sap and in the coastal provinces, and provide a geo-statistical model of arsenic in shallow groundwater for the whole country.

 
  
 

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These articles have been peer reviewed and accepted for publication. They are still in production and have not been edited, so may differ from the final published form.

    EN14138  Accepted 22 October 2014
    Hydroxyl Radical Initiated Oxidation of Formic Acid on Mineral Aerosols Surface. A Mechanistic, Kinetic and Spectroscopic Study
    Cristina Iuga, Claro SAINZ-DIAZ, Annik Vivier-Bunge
    Abstract


    EN14105  Accepted 22 October 2014
    Use of DGT for studies of chemical speciation and bioavailability
    Hao Zhang, William Davison
    Abstract


    EN14124  Accepted 17 October 2014
    The formation and fate of organoarsenic species in marine ecosystems: Do existing experimental approaches appropriately simulate ecosystem complexity?
    Elliott Duncan, Bill Maher, Simon Foster
    Abstract


    EN14135  Accepted 15 October 2014
    Comparative characterization of two fulvic acids from East lake and Liangzi lake in central China
    Jun Wang, Huijie Li, Yong Chen, Yuan Fang, Zongping Wang, Tao Tao, Yeugang Zuo
    Abstract


    EN14126  Accepted 08 October 2014
    Characterising sediments of a tropical sediment-starved continental shelf using cluster analysis of physical and geochemical variables
    Lynda Radke, Jin Li, Grant Douglas, Rachel Przeslawski, Scott Nichol, Justy Siwabessy, Zhi Huang, Janice Trafford, Tony Watson, Tanya Whiteway
    Abstract


    EN14042  Accepted 29 September 2014
    Multi-Elemental STXM-NEXAFS Assessment of Organo-Mineral Associations in Soils from Reduced Environments
    Chunmei Chen, Donald Sparks
    Abstract


    EN14129  Accepted 25 September 2014
    Characterization of Oil Contaminated Soils via Comprehensive Multiphase NMR
    Hashim Farooq, Denis Courtier-Murias, Myrna Simpson, Werner Maas, Michael Fey, Brian Andrew, Jochem Struppe, Howard Hutchins, Sridevi Krishnamurthy, Rajeev Kumar, Martine Monette, Henry Stronks, Andre Simpson
    Abstract


    EN14128  Accepted 23 September 2014
    Quantification of individual polysulfides in lab-scale and full-scale desulfurization bioreactors
    Pawel Roman, Martijn Bijmans, Albert Janssen
    Abstract


    EN14065  Accepted 22 September 2014
    Adsorption of Novel Insensitive Munitions Compounds at Clay Mineral and Metal Oxide Surfaces
    Billy Linker, Raju Khatiwada, Nico Perdrial, Leif Abrell, Reyes Sierra, James Field, Jon Chorover
    Abstract


    EN14093  Accepted 16 September 2014
    Reversible exchange of stable nitroxyl radicals on nanosilver particles
    Mark Chappell, Lesley Miller, Cynthia Price
    Abstract


    EN14116  Accepted 01 September 2014
    Degradation of Oxytetracycline in the Aquatic Environment: A proposed Steady State Kinetic Model that takes into account Hydrolysis, Photolysis, Microbial Degradation and Adsorption by Colloidal and Sediment Particles.
    Mark Zaranyika, Pamhidzai Dzomba, Jameson Kugara
    Abstract


    EN14035  Accepted 30 August 2014
    Fe(II)aq - Fe(III)oxide electron transfer and Fe exchange: Effect of organic carbon
    Timothy Pasakarnis, Michael McCormick, Gene Parkin, Aaron Thompson, Michelle Scherer
    Abstract


    EN14008  Accepted 30 August 2014
    Effect of multivalent cations, temperature, and ageing on SOM interfacial properties
    Doerte Diehl, Tatjana Schneckenburger, Jaane Krueger, Marc-Oliver Goebel, Susanne Woche, Jette Schwarz, Anastasia Shchegolikhina, Friederike Lang, Bernd Marschner, Soeren Thiele-Bruhn, Joerg Bachmann, Gabriele Schaumann
    Abstract


    EN13216  Accepted 30 August 2014
    Interpretation of Heavy Metal Speciation in Sequential Extraction Using Geochemical Modeling
    Yanshan Cui, Liping Weng
    Abstract


    EN14127  Accepted 22 August 2014
    A Critical Review of Nanohybrids: Synthesis, Applications, and Environmental Implications
    Nirupam Aich, Jaime Plazas-Tuttle, Jamie Lead, Navid Saleh
    Abstract


    EN14086  Accepted 14 August 2014
    Metal ion complexation by soft nanoparticles: the impact of Ca2+ on electrostatic and chemical contributions to the Eigen-type reaction rate
    Raewyn Town
    Abstract


    EN14123  Accepted 13 August 2014
    Antimony leaching from contaminated soil under manganese- and iron-reducing conditions: column experiments
    Kerstin Hockmann, Susan Tandy, Markus Lenz, Rainer Schulin
    Abstract


    EN13240  Accepted 12 August 2014
    Synchrotron XAS analysis of arsenic chemical speciation in human nail clippings
    Olena Ponomarenko, Mihai Gherase, Mark LeBlanc, Chang-Yong Kim, Elstan Desouza, Michael Farquharson, Fiona McNeill, Susan Nehzati, Ingrid Pickering, Graham George, David Fleming
    Abstract


    EN14045  Accepted 02 August 2014
    Geochemical Reaction Mechanism Discovery from Molecular Simulation.
    Andrew Stack, Paul Kent
    Abstract


    EN14100  Accepted 26 July 2014
    Lability of Pb in soil: effects of soil properties and contaminant source.
    Lingchen Mao, Elizabeth Bailey, Jonathan Chester, Joseph Dean, E Ander, Simon Chenery, Scott Young
    Abstract


    EN14047  Accepted 25 July 2014
    Measurement of labile arsenic speciation in water and soil using Diffusive Gradients in Thin-films (DGT) and X-ray Absorption Near Edge Spectroscopy (XANES)
    Trang Huynh, Hugh Harris, Hao Zhang, Barry Noller
    Abstract


    EN14097  Accepted 23 July 2014
    Seasonal distributions and sources of low molecular weight dicarboxylic acids, ω-oxocarboxylic acids, pyruvic acid, α-dicarbonyls and fatty acids in ambient aerosols from subtropical Okinawa in the western Pacific rim
    Bhagawati Kunwar, Kimitaka Kawamura
    Abstract


    EN14041  Accepted 21 July 2014
    Oxidation of Cr(III) Aminocarboxylate Complexes by Hydrous Manganese Oxide: Products and Time Course Behavior
    Richard Carbonaro, Alan Stone
    Abstract


    EN14068  Accepted 11 July 2014
    Interpretation of DGT measurements. Review of a systematic approach
    Josep Galceran, Jaume Puy
    Abstract


    EN14091  Accepted 30 June 2014
    Two dispersive liquid–liquid microextraction methods coupled with GC–MS for the determination of organophosphorus pesticides in field water
    Shang-Ping Chu, Chun-Kai Huang, Pai-Shan Chen, Shang-Da Huang
    Abstract


    EN14078  Accepted 28 June 2014
    Comparative analyses of cadmium and zinc uptake correlated with changes in NRAMP expression in Solanum nigrum L. and Brassica rapa
    Y Song, Lee Hudek, David Freestone, J Puhui, Agnes Michalczyk, Senlin Zheng, M Leigh Ackland
    Abstract


    EN14054  Accepted 27 June 2014
    Chemical and bioanalytical assessment of coal seam gas associated water
    Janet Tang, Mauricio Taulis, Jacinta Edebeli, Frederic Leusch, Paul Jagals, Gregory Jackson, Beate Escher
    Abstract


    EN14043  Accepted 27 May 2014
    Ligand- and oxygen-isotope-exchange pathways of geochemical interest
    Bill Casey
    Abstract




The Most Read ranking is based on the number of downloads from the CSIRO PUBLISHING website of articles published in the previous 12 months. Usage statistics are updated daily.

Rank Paper Details
1. Published 19 December 2013
Organic phosphorus in the aquatic environment

Darren S. Baldwin

2. Published 19 December 2013
Organic fluorine content in aqueous film forming foams (AFFFs) and biodegradation of the foam component 6 : 2 fluorotelomermercaptoalkylamido sulfonate (6 : 2 FTSAS)

Barbara Weiner, Leo W. Y. Yeung, Erin B. Marchington, Lisa A. D'Agostino and Scott A. Mabury

3. Published 25 February 2014
Hard X-ray synchrotron biogeochemistry: piecing together the increasingly detailed puzzle

Enzo Lombi, Ryo Sekine and Erica Donner

4. Published 19 December 2013
Predicting PbII adsorption on soils: the roles of soil organic matter, cation competition and iron (hydr)oxides

Zhenqing Shi, Herbert E. Allen, Dominic M. Di Toro, Suen-Zone Lee and James B. Harsh

5. Published 28 April 2014
Metal complexation by organic ligands (L) in near-pristine estuarine waters: evidence for the identity of L

Hollydawn Murray, Guillaume Meunier, Dagmar B. Stengel and Rachel Cave

6. Published 24 June 2014
Aquatic toxicity of manufactured nanomaterials: challenges and recommendations for future toxicity testing

Aaron G. Schultz, David Boyle, Danuta Chamot, Kimberly J. Ong, Kevin J. Wilkinson, James C. McGeer, Geoff Sunahara and Greg G. Goss

7. Published 25 February 2014
Visualising Fe speciation diversity in ocean particulate samples by micro X-ray absorption near-edge spectroscopy

Matthew A. Marcus and Phoebe J. Lam

8. Published 25 October 2013
Composition of water-soluble organic carbon in non-urban atmospheric aerosol collected at the Storm Peak Laboratory

Vera Samburova, A. Gannet Hallar, Lynn R. Mazzoleni, Parichehr Saranjampour, Douglas Lowenthal, Steven D. Kohl and Barbara Zielinska

9. Published 28 April 2014
A critical look at the calculation of the binding characteristics and concentration of iron complexing ligands in seawater with suggested improvements

Loes J. A. Gerringa, Micha J. A. Rijkenberg, Charles-Edouard Thuróczy and Leo R. M. Maas

10. Published 25 February 2014
Effect of biogeochemical redox processes on the fate and transport of As and U at an abandoned uranium mine site: an X-ray absorption spectroscopy study

Lyndsay D. Troyer, James J. Stone and Thomas Borch

11. Published 28 April 2014
Voltammetric characterisation of macroalgae-exuded organic ligands (L) in response to Cu and Zn: a source and stimuli for L

Hollydawn Murray, Guillaume Meunier, Constant M. G. van den Berg, Rachel R. Cave and Dagmar B. Stengel

12. Published 24 June 2014
Speciation mapping of environmental samples using XANES imaging

Barbara E. Etschmann, Erica Donner, Joël Brugger, Daryl L. Howard, Martin D. de Jonge, David Paterson, Ravi Naidu, Kirk G. Scheckel, Chris G. Ryan and Enzo Lombi

13. Published 19 December 2013
Bauxite residue neutralisation precipitate stability in acidic environments

Sara J. Couperthwaite, Sujung Han, Talitha Santini, Gurkiran Kaur, Dean W. Johnstone, Graeme J. Millar and Ray L. Frost

14. Published 25 October 2013
Secondary organic aerosol tracers and malic acid in Hong Kong: seasonal trends and origins

Di Hu and Jian Zhen Yu

15. Published 25 February 2014
Environmental chemistry: a discipline standing on two shoulders

Montserrat Filella

16. Published 25 February 2014
Scaling up: fulfilling the promise of X-ray microprobe for biogeochemical research

Brandy M. Toner, Sarah L. Nicholas and Jill K. Coleman Wasik

17. Published 24 June 2014
The influence of particle size and structure on the sorption and oxidation behaviour of birnessite: II. Adsorption and oxidation of four polycyclic aromatic hydrocarbons

Mario Villalobos, Manuel Carrillo-Cárdenas, Richard Gibson, N. Ruth López-Santiago and Jimmy A. Morales

18. Published 25 February 2014
Diffusion limitation of zinc fluxes into wheat roots, PLM and DGT devices in the presence of organic ligands

A. Gramlich, S. Tandy, E. Frossard, J. Eikenberg and R. Schulin

19. Published 25 February 2014
Synchrotron X-ray distinction of seasonal hydrological and temperature patterns in speleothem carbonate

Peter M. Wynn, Ian J. Fairchild, Christoph Spötl, Adam Hartland, Dave Mattey, Barbara Fayard and Marine Cotte

20. Published 25 October 2013
Combination of nitrate (N, O) and boron isotopic ratios with microbiological indicators for the determination of nitrate sources in karstic groundwater

Cyrielle Briand, Valérie Plagnes, Mathieu Sebilo, Pascale Louvat, Thierry Chesnot, Maude Schneider, Pierre Ribstein and Pierre Marchet


      
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