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Contents Vol 65(7)

The Chemistry of Transition Metal Ethyne-1,2-diyl Complexes*

Christopher S. Griffith A B and George A. Koutsantonis A C
+ Author Affiliations
- Author Affiliations

A Chemistry, M313, School of Chemistry and Biochemistry, University of Western Australia, Crawley, Perth, WA 6009, Australia.

B Present address: ANSTO Minerals, Australian Nuclear Science and Technology Organisation, Locked Bag 2001 Kirrawee DC, NSW 2232, Australia.

C Corresponding author. Email: george.koutsantonis@uwa.edu.au




Dr Christopher S. Griffith is a Senior Process Chemist at the Australian Nuclear Science and Technology Organisation (ANSTO) Minerals business unit. He is currently involved with numerous commercial research projects for the uranium, rare-earth industries and industries in which naturally occurring radioactive material (NORM) are present. Dr Griffith has 10 years of experience working in the research and development of hydrometallurgical and pyrometallurgical separation technologies, applicable to current and advanced nuclear fuel cycles. He completed his PhD in Chemistry at the University of Western Australia in 2000 studying the synthesis and reactivity of Group 8 ethyne-1,2-diyl complexes with George Koutsantonis. He has over 35 peer reviewed publications, over 50 commercial-in-confidence technical reports, and over 20 international conference publications.


George A. Koutsantonis is a synthetic chemist with an interest in functional materials that contain metals. He is a graduate of the University of Adelaide and began his scientific life studying the coordination properties and reactions of alkynes and often returns to this fascinating area. He was appointed to the staff at the University of Western Australia in 1995 where he remains. The work in this detailed review was recognised by the joint RACI Organometallic award in 2004. He is indebted to his co-author for all his efforts in expanding the chemistry of ethyndiyl complexes.

Australian Journal of Chemistry 65(7) 698-722 https://doi.org/10.1071/CH12190
Submitted: 10 April 2012  Accepted: 18 June 2012   Published: 2 August 2012

Abstract

The chemistry and reactivity of ethyne-1,2-diyl compounds, LnM–CC–MLn, is reviewed. These complexes are simple analogues of organic alkynes, or dimetalloalkynes, and there appears to be no general route to the preparation of these complexes, except perhaps using acid/base methodology. Reactivity patterns, in general, mimic those of simple organic alkynes but have the added dimension of reactive M–C(sp) bonds that sometimes participate in the formation of multimetallic compounds with metal electrophiles.


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