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Open Access Article << Previous     |     Next >>   Contents Vol 65(8)

Living Radical Polymerization by the RAFT Process – A Third Update

Graeme Moad A B , Ezio Rizzardo A and San H. Thang A

A CSIRO Materials Science and Engineering, Bag 10, Clayton South, Vic. 3169, Australia.
B Corresponding author. Email: graeme.moad@csiro.au

Australian Journal of Chemistry 65(8) 985-1076 http://dx.doi.org/10.1071/CH12295
Submitted: 19 June 2012  Accepted: 25 July 2012   Published: 7 September 2012


 
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Abstract

This paper provides a third update to the review of reversible deactivation radical polymerization (RDRP) achieved with thiocarbonylthio compounds (ZC(=S)SR) by a mechanism of reversible addition-fragmentation chain transfer (RAFT) that was published in June 2005 (Aust. J. Chem. 2005, 58, 379). The first update was published in November 2006 (Aust. J. Chem. 2006, 59, 669) and the second in December 2009 (Aust. J. Chem. 2009, 62, 1402). This review cites over 700 publications that appeared during the period mid 2009 to early 2012 covering various aspects of RAFT polymerization which include reagent synthesis and properties, kinetics and mechanism of polymerization, novel polymer syntheses, and a diverse range of applications. This period has witnessed further significant developments, particularly in the areas of novel RAFT agents, techniques for end-group transformation, the production of micro/nanoparticles and modified surfaces, and biopolymer conjugates both for therapeutic and diagnostic applications.





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